Stability of plasmonic metal nanoparticles integrated in the back contact of ultra-thin Cu(In,Ga)S2 solar cells
Identifieur interne : 000499 ( Main/Repository ); précédent : 000498; suivant : 000500Stability of plasmonic metal nanoparticles integrated in the back contact of ultra-thin Cu(In,Ga)S2 solar cells
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Abstract
Ultra-thin solar cells on transparent back contacts constitute the basis for highly efficient tandem solar devices which can surpass the single cell efficiency limit. The material reduction related to ultra-thin high efficiency devices additionally lowers the price. Despite the fact that they are ultra-thin the absorbers still have to remain optically thick and therefore require adequate light management. A promising approach for enhanced absorption is plasmonic scattering from metal nanoparticles. In this paper we discuss the experimental incorporation of Ag nanoparticles in ultra-thin wide-gap chalcopyrite solar cells on transparent back contacts. A 6.9% efficient 500 nm Cu(In,Ga)S2 solar cell on In2O3:Mo (at this point without nanoparticles) is the starting point. For the predicted optimum design of including particles at the rear side the stability of the nanostructures integrated in the back contact is investigated in detail. As a first step towards proof-of-concept, absorption enhancement from the nanoparticles included in the complete solar cell is experimentally shown in optical properties.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Stability of plasmonic metal nanoparticles integrated in the back contact of ultra-thin Cu(In,Ga)S<sub>2</sub> solar cells</title><author><name sortKey="Schmid, M" uniqKey="Schmid M">M. Schmid</name><affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Helmholtz Zentrum Berlin, Heterogeneous Material Systems, Hahn-Meitner-Platz 1</s1><s2>14109 Berlin</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="3">Berlin</region><settlement type="city">Berlin</settlement></placeName></affiliation></author><author><name sortKey="Klaer, J" uniqKey="Klaer J">J. Klaer</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Helmholtz Zentrum Berlin, Technology, Hahn-Meitner-Platz 1</s1><s2>14109 Berlin</s2><s3>DEU</s3><sZ>2 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="3">Berlin</region><settlement type="city">Berlin</settlement></placeName></affiliation></author><author><name sortKey="Klenk, R" uniqKey="Klenk R">R. Klenk</name><affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Helmholtz Zentrum Berlin, Heterogeneous Material Systems, Hahn-Meitner-Platz 1</s1><s2>14109 Berlin</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="3">Berlin</region><settlement type="city">Berlin</settlement></placeName></affiliation></author><author><name sortKey="Topic, M" uniqKey="Topic M">M. Topic</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>University of Ljubljana, Faculty of Electrical Engineering, Tržaška 25</s1><s2>1000 Ljubljana</s2><s3>SVN</s3><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>Slovénie</country><wicri:noRegion>1000 Ljubljana</wicri:noRegion></affiliation></author><author><name sortKey="Krc, J" uniqKey="Krc J">J. Krc</name><affiliation wicri:level="1"><inist:fA14 i1="03"><s1>University of Ljubljana, Faculty of Electrical Engineering, Tržaška 25</s1><s2>1000 Ljubljana</s2><s3>SVN</s3><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>Slovénie</country><wicri:noRegion>1000 Ljubljana</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="inist">13-0132050</idno><date when="2013">2013</date><idno type="stanalyst">PASCAL 13-0132050 INIST</idno><idno type="RBID">Pascal:13-0132050</idno><idno type="wicri:Area/Main/Corpus">001029</idno><idno type="wicri:Area/Main/Repository">000499</idno></publicationStmt><seriesStmt><idno type="ISSN">0040-6090</idno><title level="j" type="abbreviated">Thin solid films</title><title level="j" type="main">Thin solid films</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Chalcopyrite</term><term>Copper</term><term>Gallium</term><term>Indium oxide</term><term>Nanoparticles</term><term>Nanostructured materials</term><term>Nanostructures</term><term>Optical properties</term><term>Plasmons</term><term>Rapid thermal processing</term><term>Silver</term><term>Solar cells</term><term>Thin films</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Plasmon</term><term>Nanoparticule</term><term>Nanomatériau</term><term>Cellule solaire</term><term>Nanostructure</term><term>Propriété optique</term><term>Couche mince</term><term>Traitement thermique rapide</term><term>Cuivre</term><term>Gallium</term><term>Argent</term><term>Chalcopyrite</term><term>Oxyde d'indium</term><term>Substrat Molybdène</term><term>In2O3</term><term>8107</term><term>8460J</term><term>7866</term></keywords><keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Cuivre</term><term>Argent</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Ultra-thin solar cells on transparent back contacts constitute the basis for highly efficient tandem solar devices which can surpass the single cell efficiency limit. The material reduction related to ultra-thin high efficiency devices additionally lowers the price. Despite the fact that they are ultra-thin the absorbers still have to remain optically thick and therefore require adequate light management. A promising approach for enhanced absorption is plasmonic scattering from metal nanoparticles. In this paper we discuss the experimental incorporation of Ag nanoparticles in ultra-thin wide-gap chalcopyrite solar cells on transparent back contacts. A 6.9% efficient 500 nm Cu(In,Ga)S<sub>2</sub> solar cell on In<sub>2</sub>O<sub>3</sub>:Mo (at this point without nanoparticles) is the starting point. For the predicted optimum design of including particles at the rear side the stability of the nanostructures integrated in the back contact is investigated in detail. As a first step towards proof-of-concept, absorption enhancement from the nanoparticles included in the complete solar cell is experimentally shown in optical properties.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0040-6090</s0></fA01><fA02 i1="01"><s0>THSFAP</s0></fA02><fA03 i2="1"><s0>Thin solid films</s0></fA03><fA05><s2>527</s2></fA05><fA08 i1="01" i2="1" l="ENG"><s1>Stability of plasmonic metal nanoparticles integrated in the back contact of ultra-thin Cu(In,Ga)S<sub>2</sub> solar cells</s1></fA08><fA11 i1="01" i2="1"><s1>SCHMID (M.)</s1></fA11><fA11 i1="02" i2="1"><s1>KLAER (J.)</s1></fA11><fA11 i1="03" i2="1"><s1>KLENK (R.)</s1></fA11><fA11 i1="04" i2="1"><s1>TOPIC (M.)</s1></fA11><fA11 i1="05" i2="1"><s1>KRC (J.)</s1></fA11><fA14 i1="01"><s1>Helmholtz Zentrum Berlin, Heterogeneous Material Systems, Hahn-Meitner-Platz 1</s1><s2>14109 Berlin</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>3 aut.</sZ></fA14><fA14 i1="02"><s1>Helmholtz Zentrum Berlin, Technology, Hahn-Meitner-Platz 1</s1><s2>14109 Berlin</s2><s3>DEU</s3><sZ>2 aut.</sZ></fA14><fA14 i1="03"><s1>University of Ljubljana, Faculty of Electrical Engineering, Tržaška 25</s1><s2>1000 Ljubljana</s2><s3>SVN</s3><sZ>4 aut.</sZ><sZ>5 aut.</sZ></fA14><fA20><s1>308-313</s1></fA20><fA21><s1>2013</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>13597</s2><s5>354000503724660530</s5></fA43><fA44><s0>0000</s0><s1>© 2013 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>23 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>13-0132050</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Thin solid films</s0></fA64><fA66 i1="01"><s0>NLD</s0></fA66><fC01 i1="01" l="ENG"><s0>Ultra-thin solar cells on transparent back contacts constitute the basis for highly efficient tandem solar devices which can surpass the single cell efficiency limit. The material reduction related to ultra-thin high efficiency devices additionally lowers the price. Despite the fact that they are ultra-thin the absorbers still have to remain optically thick and therefore require adequate light management. A promising approach for enhanced absorption is plasmonic scattering from metal nanoparticles. In this paper we discuss the experimental incorporation of Ag nanoparticles in ultra-thin wide-gap chalcopyrite solar cells on transparent back contacts. A 6.9% efficient 500 nm Cu(In,Ga)S<sub>2</sub> solar cell on In<sub>2</sub>O<sub>3</sub>:Mo (at this point without nanoparticles) is the starting point. For the predicted optimum design of including particles at the rear side the stability of the nanostructures integrated in the back contact is investigated in detail. 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